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Abstract The increasing integration of Visual Language Models (VLMs) into visualization systems demands a comprehensive understanding of their visual interpretation capabilities and constraints. While existing research has examined individual models, systematic comparisons of VLMs' visualization literacy remain unexplored. We bridge this gap through a rigorous, first‐of‐its‐kind evaluation of four leading VLMs (GPT‐4, Claude, Gemini, and Llama) using standardized assessments: the Visualization Literacy Assessment Test (VLAT) and Critical Thinking Assessment for Literacy in Visualizations (CALVI). Our methodology uniquely combines randomized trials with structured prompting techniques to control for order effects and response variability ‐ a critical consideration overlooked in many VLM evaluations. Our analysis reveals that while specific models demonstrate competence in basic chart interpretation (Claude achieving 67.9% accuracy on VLAT), all models exhibit substantial difficulties in identifying misleading visualization elements (maximum 30.0% accuracy on CALVI). We uncover distinct performance patterns: strong capabilities in interpreting conventional charts like line charts (76‐96% accuracy) and detecting hierarchical structures (80‐100% accuracy), but consistent difficulties with data‐dense visualizations involving multiple encodings (bubble charts: 18.6‐61.4%) and anomaly detection (25‐30% accuracy). Significantly, we observe distinct uncertainty management behavior across models, with Gemini displaying heightened caution (22.5% question omission) compared to others (7‐8%). These findings provide crucial insights for the visualization community by establishing reliable VLM evaluation benchmarks, identifying areas where current models fall short, and highlighting the need for targeted improvements in VLM architectures for visualization tasks. To promote reproducibility, encourage further research, and facilitate benchmarking of future VLMs, our complete evaluation framework, including code, prompts, and analysis scripts, is available athttps://github.com/washuvis/VisLit‐VLM‐Eval.